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Mechanistic studies on the catalytic cycle of metal fluoride-catalyzed allylation using allyltrimethoxysilane in protic solvents

ISSN:0022-3263
2003年第68卷第19期
Aoyama N,Hamada T,Manabe K,Kobayashi S Aoyama Naohiro,Hamada Tomoaki,Manabe Kei,Kobayashi Shū


The catalytic cycles of CdF(2).1-catalyzed and AgF.BINAP-catalyzed allylation using allyltrimethoxysilane in protic solvents were investigated. The experimental and (19)F NMR studies strongly supported that metal fluorides were regenerated from silyl fluoride species, and that these reactions were truly fluoride-catalyzed reactions. It was revealed that these catalytic cycles were much different from that of TBAF-catalyzed allylation using allyltrimethylsilane in THF.

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ISSN:0022-3263
2003年第68卷第19期

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